I love all the albums. I love Shpongle. You'll just have to end up listening to all their works. None of them are boring. Hard to say but I can tell you which songs stand out the most for me:
Are You Shpongled?-Shpongle Falls
-Divine Moments of Truth (a no-brainer really; why else are we all here?!)
-...and the Day Turned to Night (amazing trip into blissfulness no matter what substance you're high on)
Divine Moments of Truth-Divine Moments of Truth [Instrumental Remix]
-Divine Moments of Truth [Shpongle Trance Remix]
-Divine Moments of Truth [Original Russian Bootleg Mix] (only true Shpongle fans will get this one
)
Tales of the Inexpressible-Dorset Perception (you can't hate this song)
-A New Way to Say "Hooray!"
-Once Upon the Sea of Blissful Awareness (drifted off in the first few seconds of the song the first time I heard it...amazing)
-Around the World in a Tea Daze
-Flute Fruit
Remixed-Dorset Perception [Total Eclipse Remix] (chilled out version of an AWESOME track)
-Around the World in a Tea Daze [Ott Remix]
-Once Upon the Sea of Blissful Awareness [Esionjim Remix]
Nothing Lasts... But Nothing Is Lost-Outer Shpongolia
-Periscopes of Consciousness + Schmaltz Herring (weird at first but definitely kicks it up later)
-...But Nothing Is Lost
-When Shall I Be Free? + The Stamen of the Shamen
-Invocation
-Molecular Superstructure
-Turn Up The Silence
-Exhalation
Unreleased Remixes-Dorset Perception [Gaudi Remix] (Another kick-ass remix of an AWESOME track)
-Dorset Perception [Lo-Step Balearic Breaks Re-Edit] (this one almost sounds the same as the original only it has a higher tone to it and the beats are a bit different)
-Periscopes of Consciousness [Greg Hunter Edit] (basically it's Periscopes of Consciousness+Schmaltz Herring mixed together in a seamless fashion to sound like a single track with added effects)
Ineffable Mysteries From Shpongleland (honestly my least favorite album because it seems to be the only one constricted to one type of musical influence [eastern/indian] but still worth a listen)
-Electroplasm
-Nothing Is Something Worth Doing
-Ineffable Mysteries
-I Am You
The God Particle EP-Before the Big Bang
-The God Particle
That pretty much sums my opinion. In the end, you're just going to have to listen to all the albums in complete,
GAPLESS playback, in order. Remember, the albums are one single track divided into sections so you can't exactly press the shuffle button and listen to them in any order. The end of the one track is the beginning of the next one....Go get Shpongled my friend!